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Life Cycle Assessment and Life Cycle Cost of an Innovative Carbon Paper Sensor for 17α-Ethinylestradiol and Comparison with the Classical Chromatographic Method

2022-07-20Journal article Open access
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dc.contributor.authorMartins, Florinda
dc.contributor.authorTorrinha, Álvaro
dc.contributor.authorDelerue-Matos, Cristina
dc.contributor.authorMorais, Simone
dc.date.accessioned2023-01-31T10:25:42Z
dc.date.available2023-01-31T10:25:42Z
dc.date.issued2022-07-20
dc.description.abstractNowadays there is a growing concern with the environment and sustainability, which means that better methods, including pollutants analysis, with less consumption of materials, organic solvents, and energy, need to be developed. Considering the almost inexistent information about the topic, the main goal of this work was to compare the environmental impacts of two analytical methods, a traditional one based on liquid chromatography with fluorescence detection and a newly developed carbon paper sensor. The selected analyte was 17α-ethinylestradiol, which is a contaminant of emergent concern in aquatic ecosystems due to its endocrine disruptor behavior. The life cycle assessment data showed that the sensor detection presents an almost negligible environmental impact when compared with the extraction step (the same for both methods) and the liquid chromatographic determination (roughly 80 times higher than with the sensor). The sensor values for all categories of damage are below 3% of the total method impacts, i.e., 1.6, 1.9, 2.4, and 2.9% for resources, climate change, human health, and ecosystem quality. The extraction represents 98.1% of the sensor environmental impacts (and 99.6% of its life cycle costing) and 38.8% of the chromatographic method. This study evidences the need of developing and applying greener analytical (detection and extraction) strategiespt_PT
dc.description.sponsorshipThis work was financed by FEDER—Fundo Europeu de Desenvolvimento Regional funds through the COMPETE 2020—Operacional Programme for Competitiveness and Internationalization (POCI), and by Portuguese funds through FCT—Fundação para a Ciência e a Tecnologia in the framework of the project POCI-01-0145-FEDER-029547—PTDC/ASP-PES/29547/2017. This work received support by UIDB/50006/2020, UIDP/50006/2020 and LA/P/0008/2020 by the Fundação para a Ciência e a Tecnologia (FCT), Ministério da Ciência, Tecnologia e Ensino Superior (MCTES) through national funds.pt_PT
dc.description.versioninfo:eu-repo/semantics/publishedVersionpt_PT
dc.identifier.doi10.3390/su14148896pt_PT
dc.identifier.urihttp://hdl.handle.net/10400.22/22023
dc.language.isoengpt_PT
dc.publisherMDPIpt_PT
dc.relationLA/P/0008/2020pt_PT
dc.relation(Bio)sensors for assessment of contaminants of emerging concern in fishery commodities
dc.relationAssociated Laboratory for Green Chemistry - Clean Technologies and Processes
dc.relationAssociated Laboratory for Green Chemistry - Clean Technologies and Processes
dc.relation.publisherversionhttps://www.mdpi.com/2071-1050/14/14/8896pt_PT
dc.rights.urihttp://creativecommons.org/licenses/by-nc-nd/4.0/pt_PT
dc.subjectCarbon paperpt_PT
dc.subjectChromatographypt_PT
dc.subjectContaminants of emerging concernpt_PT
dc.subjectElectroanalysispt_PT
dc.subjectEthinylestradiolpt_PT
dc.subjectGreen analytical chemistrypt_PT
dc.subjectLife cycle assessmentpt_PT
dc.subjectLife cycle costpt_PT
dc.subjectSensorpt_PT
dc.titleLife Cycle Assessment and Life Cycle Cost of an Innovative Carbon Paper Sensor for 17α-Ethinylestradiol and Comparison with the Classical Chromatographic Methodpt_PT
dc.typejournal article
dspace.entity.typePublication
oaire.awardTitle(Bio)sensors for assessment of contaminants of emerging concern in fishery commodities
oaire.awardTitleAssociated Laboratory for Green Chemistry - Clean Technologies and Processes
oaire.awardTitleAssociated Laboratory for Green Chemistry - Clean Technologies and Processes
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/9471 - RIDTI/PTDC%2FASP-PES%2F29547%2F2017/PT
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/6817 - DCRRNI ID/UIDB%2F50006%2F2020/PT
oaire.awardURIinfo:eu-repo/grantAgreement/FCT/6817 - DCRRNI ID/UIDP%2F50006%2F2020/PT
oaire.citation.issue14pt_PT
oaire.citation.startPage8896pt_PT
oaire.citation.titleSustainabilitypt_PT
oaire.citation.volume14pt_PT
oaire.fundingStream9471 - RIDTI
oaire.fundingStream6817 - DCRRNI ID
oaire.fundingStream6817 - DCRRNI ID
person.familyNameMartins
person.familyNameTorrinha
person.familyNameDelerue-Matos
person.familyNameMorais
person.givenNameF.
person.givenNameÁlvaro
person.givenNameCristina
person.givenNameSimone
person.identifier1495443
person.identifier1598822
person.identifier.ciencia-id2D1F-FFB3-34B8
person.identifier.ciencia-id9A1A-43FB-5C27
person.identifier.ciencia-idB111-BBFB-F200
person.identifier.orcid0000-0002-8866-1799
person.identifier.orcid0000-0002-9829-8559
person.identifier.orcid0000-0002-3924-776X
person.identifier.orcid0000-0001-6433-5801
person.identifier.ridD-4990-2013
person.identifier.scopus-author-id56060519600
person.identifier.scopus-author-id6603741848
person.identifier.scopus-author-id7007053747
project.funder.identifierhttp://doi.org/10.13039/501100001871
project.funder.identifierhttp://doi.org/10.13039/501100001871
project.funder.identifierhttp://doi.org/10.13039/501100001871
project.funder.nameFundação para a Ciência e a Tecnologia
project.funder.nameFundação para a Ciência e a Tecnologia
project.funder.nameFundação para a Ciência e a Tecnologia
rcaap.rightsopenAccesspt_PT
rcaap.typearticlept_PT
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